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Regioselective addition of Grignard reagents to N -acylpyrazinium salts: synthesis of substituted 1,2-dihydropyrazines and Δ 5 -2-oxopiperazines.
The regioselective addition of Grignard reagents to mono- and disubstituted N -acylpyrazinium salts affording substituted 1,2-dihydropyrazines in modest to excellent yields (45-100%) is described. Under acidic conditions, these 1,2-dihydropyrazines can be converted to substituted Δ5 -2-oxopiperazines providing a simple and efficient approach towards their preparation.
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