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A highly enantioselective asymmetric Darzens reaction catalysed by proline based efficient organocatalysts for the synthesis of di- and tri-substituted epoxides.
Chemical Communications : Chem Comm 2017 October 4
A new class of easily available and readily tunable proline based chiral organocatalysts was found to efficiently catalyse an unprecedented highly enantioselective asymmetric Darzens reaction of α-chloroketones and substituted α-chloroketones with various aldehydes, which directly produces optically active di- and tri-substituted chiral epoxides with higher product yields (up to 97%) and excellent ee's (up to 99%) under mild reaction conditions.
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