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Recent progress in development of molecular catalyst-based anodes for water oxidation toward artificial photosynthesis.
ChemSusChem 2019 Februrary 22
Catalytic water oxidation represents the bottleneck for developing artificial photosynthetic systems that store solar energy as renewable fuels. A variety of molecular water oxidation catalysts (WOCs) were reported over the last two decades. In view of their applications to artificial photosynthetic devices, it is essential to immobilize molecular catalysts onto surfaces of conducting/semiconducting supports for fabricating efficient and stable water oxidation anodes/photoanodes. Molecular WOC based- anodes are essential for developing the photovoltaic (PV) type of artificial photosynthetic devices and, otherwise, the performance of molecular WOC on anodes will provide important insight into designing the extended molecular WOC-based photoanodes for photoelectrochemical (PEC) water oxidation. Herein we mainly review the recent progress in the molecular WOC-based anodes over the last two decades and will look to perspective in the anodes toward artificial photosynthesis.
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