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Electrochemical Reduction of CO 2 on Hollow Cubic Cu 2 O@Au Nanocomposites.
Nanoscale Research Letters 2019 Februrary 22
Surfactant-free and low Au loading Cu2 O@Au and Au hollow cubes, based on electrodeposited Cu2 O cubes as sacrificed templates, were prepared by means of a galvanic replacement reaction (GRR). The electrocatalytical performance of the as-prepared catalysts towards carbon dioxide (CO2 ) electrochemical reduction was evaluated. The experimental results show that Cu2 O@Au catalyst can convert CO2 to carbon monoxide (CO) with a maximum Faradaic efficiency (FE) of ~ 30.1% at the potential of - 1.0 V (vs. RHE) and is about twice the FE of the other catalysts at the same potential. By comparison, such electrocatalytical enhancement is attributed to the metal-oxide interface in Cu2 O@Au.
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