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Tunable Topological State, High Hole-Carrier Mobility and Prominent Sunlight Absorbance in Monolayered Calcium Triarsenide.
Journal of Physical Chemistry Letters 2019 Februrary 5
Designing novel two-dimensional (2D) materials is highly desirable for the material innovation. Here, we proposed the monolayered calcium triarsenide (1L CaAs3) as a new 2D semiconductor with a series of encouraging functionalities. Contrast to ~33 meV small bandgap in bulk CaAs3, 1L CaAs3 possesses a large direct band gap of 0.92 eV with a high hole mobility of ~104 cm2 v1 s1. The electronic properties of 2D CaAs3 can be manipulated significantly by the layer thickness and external strains. Remarkably, 2D CaAs3 suggests a topologically nontrivial-trivial states transition under thickness reduction and strain engineering, which is attributed to the drastic surface relaxation and pinch-effect under compression. A semiconductor-semimetal transition is also revealed when the layer thickness is more than 3L. Furthermore, 1L CaAs3 exhibits prominent visible-light absorption compared with the crystalline silicon. All these desired properties render 2D CaAs3 a promising candidate in the electronic and photovoltaic devices.
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