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Efficient photon upconversion at remarkably low annihilator concentrations in a liquid polymer matrix: when less is more.
Chemical Communications : Chem Comm 2018 November 30
A green-to-blue triplet-triplet annihilation upconversion of 24.5% quantum yield was achieved at a remarkably low 600 μM annihilator concentration in a viscous polymer matrix. This was made possible by utilizing a ZnTPP-based photosensitizer with exceptionally long 11 ms phosphorescence lifetime. Higher 3 mM annihilator concentration resulted in lower 24% upconversion quantum yield.
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