Adjustable exciton-photon coupling with giant Rabi-splitting using layer-by-layer J-aggregate thin films in all-metal mirror microcavities

Hung-Sen Wei, Cheng-Chung Jaing, Yan-Ting Chen, Chen-Chih Lin, Ching-Wei Cheng, Chia-Hua Chan, Cheng-Chung Lee, Jui-Fen Chang
Optics Express 2013 September 9, 21 (18): 21365-73
Developing of highly absorbing thin films is essential for exploration of light-matter interaction and polariton-based applications. We demonstrate here layer-by-layer assembled J-aggregate thin films of (DEDOC) cyanine dyes that have high absorption coefficient and controlled thicknesses, leading to adjustable exciton-photon coupling and Rabi splitting exceeding 400 meV at room temperature in all-metal mirror microcavities.

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