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JOURNAL ARTICLE
RESEARCH SUPPORT, NON-U.S. GOV'T
Helical growth of semiconducting columnar dye assemblies based on chiral perylene bisimides.
Organic Letters 2007 March 16
A perylene bisimide derivative bearing two phenyl substituents with chiral solubilizing alkyl chains at the imide N atoms has been synthesized, and its self-assembly properties in solution and condensed phase have been investigated. Temperature-dependent CD spectra revealed the coexistence of two different kinds of chiral aggregates, differing in size and handedness. The chiral side chains effect a higher order within the self-assemblies, resulting in an increased charge-carrier mobility in the columnar liquid crystalline mesophase. [structure: see text]
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