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https://read.qxmd.com/read/30785717/in-silico-design-and-characterization-of-graphene-oxide-membranes-with-variable-water-content-and-flake-oxygen-content
#1
Christopher D Williams, Paola Carbone, Flor R Siperstein
Graphene oxide (GO) membranes offer exceptional promise for certain aqueous separation challenges, such as desalination. Central to unlocking this promise and optimising performance for a given separation is the establishment of a detailed molecular-level understanding of how the membrane's composition affects its structural and transport properties. This understanding is currently lacking, in part due to the fact that, until recently, molecular models with a realistic distribution of oxygen-functionalities and interlayer flake structure were unavailable...
February 20, 2019: ACS Nano
https://read.qxmd.com/read/30782366/ptni-bimetallic-nanoparticles-loaded-mos-2-nanosheets-preparation-and-electrochemical-sensing-application-for-the-detection-of-dopamine-and-uric-acid
#2
Lian Ma, Qiaran Zhang, Chao Wu, Yue Zhang, Lintao Zeng
Composite nanomaterials are particularly useful and offer many excellent opportunities for electrochemical sensing application. Depending on the high catalytic activity of bimetallic nanoparticles, the large specific surface area, abundant active edges and co-catalytic function of MoS2 nanosheets, we, for the first time, prepared a novel PtNi bimetallic nanoparticles loaded MoS2 nanosheets (PtNi@MoS2 ) hybrid material by a co-reduction method for the electrochemical sensing application. The nanocomposite is characterized by scanning electron microscopy (SEM), X-ray diffraction (XRD), energy dispersive spectroscopy (EDS) and X-ray photoelectron spectroscopy (XPS), and then casted on a bare glassy carbon electrode (GCE) to fabricate an electrochemical sensor (PtNi@MoS2 /GCE)...
May 9, 2019: Analytica Chimica Acta
https://read.qxmd.com/read/30781545/electrospinning-of-polystyrene-polyhydroxybutyrate-nanofibers-doped-with-porphyrin-and-graphene-for-chemiresistor-gas-sensors
#3
Joshua Avossa, Roberto Paolesse, Corrado Di Natale, Emiliano Zampetti, Giovanni Bertoni, Fabrizio De Cesare, Giuseppe Scarascia-Mugnozza, Antonella Macagnano
Structural and functional properties of polymer composites based on carbon nanomaterials are so attractive that they have become a big challenge in chemical sensors investigation. In the present study, a thin nanofibrous layer, comprising two insulating polymers (polystyrene (PS) and polyhydroxibutyrate (PHB)), a known percentage of nanofillers of mesoporous graphitized carbon (MGC) and a free-base tetraphenylporphyrin, was deposited onto an Interdigitated Electrode (IDE) by electrospinning technology. The potentials of the working temperature to drive both the sensitivity and the selectivity of the chemical sensor were studied and described...
February 17, 2019: Nanomaterials
https://read.qxmd.com/read/30781452/chitosan-based-carbon-quantum-dots-for-biomedical-applications-synthesis-and-characterization
#4
Łukasz Janus, Marek Piątkowski, Julia Radwan-Pragłowska, Dariusz Bogdał, Dalibor Matysek
Rapid development in medicine and pharmacy has created a need for novel biomaterials with advanced properties such as photoluminescence, biocompability and long-term stability. The following research deals with the preparation of novel types of N -doped chitosan-based carbon quantum dots. Nanomaterials were obtained with simultaneous nitrogen-doping using biocompatible amino acids according to Green Chemistry principles. For the carbon quantum dots synthesis chitosan was used as a raw material known for its biocompability...
February 16, 2019: Nanomaterials
https://read.qxmd.com/read/30778158/effect-of-iron-overload-from-multi-walled-carbon-nanotubes-on-neutrophil-like-differentiated-hl-60-cells
#5
Yosuke Tabei, Hiroko Fukui, Ayako Nishioka, Yuji Hagiwara, Kei Sato, Tadashi Yoneda, Tamami Koyama, Masanori Horie
Multi walled carbon nanotubes (MWCNTs) are one of the most intensively explored nanomaterials because of their unique physical and chemical properties. Due to the widespread use of MWCNTs, it is important to investigate their effects on human health. The precise mechanism of MWCNT toxicity has not been fully elucidated. The present study was designed to examine the mechanisms of MWCNT toxicity toward human promyelocytic leukemia HL-60 cells. First, we found that MWCNTs decreased the viability of neutrophil-like differentiated HL-60 cells but not undifferentiated HL-60 cells...
February 18, 2019: Scientific Reports
https://read.qxmd.com/read/30778111/immobilization-of-peroxidase-on-functionalized-mwcnts-buckypaper-polyvinyl-alcohol-nanocomposite-membrane
#6
Lau Yien Jun, N M Mubarak, Lau Sie Yon, Chua Han Bing, Mohammad Khalid, Priyanka Jagadish, E C Abdullah
Surface modified Multi-walled carbon nanotubes (MWCNTs) Buckypaper/Polyvinyl Alcohol (BP/PVA) composite membrane was synthesized and utilized as support material for immobilization of Jicama peroxidase (JP). JP was successfully immobilized on the BP/PVA membrane via covalent bonding by using glutaraldehyde. The immobilization efficiency was optimized using response surface methodology (RSM) with the face-centered central composite design (FCCCD) model. The optimum enzyme immobilization efficiency was achieved at pH 6, with initial enzyme loading of 0...
February 18, 2019: Scientific Reports
https://read.qxmd.com/read/30773721/progress-and-prospects-of-graphdiyne-based-materials-in-biomedical-applications
#7
REVIEW
Jiaming Liu, Chunying Chen, Yuliang Zhao
Graphdiyne is a new member of the family of carbon-based nanomaterials that possess two types of carbon atoms, sp- and sp2 -hybridized carbon atoms. As a novel 2D carbon-based nanomaterial with unique planar structure, such as uniformly distributed nanopores and large conjugated structure, graphdiyne has shown many fascinating properties in mechanics, electronics, and optics since it was first experimentally synthesized in 2010. Up to now, graphdiyne and its derivatives have been reported to be successfully applied in many areas, such as catalysis, energy, environment, and biomedicine, due to these excellent properties...
February 18, 2019: Advanced Materials
https://read.qxmd.com/read/30772693/facile-synthesis-of-novel-carbon-dots-hemin-nanoplatforms-for-synergistic-photo-thermal-and-photo-dynamic-therapies
#8
Wei Yang, Bing Wei, Zheng Yang, Liangquan Sheng
Due to the traditional therapies of cancer inducing huge pains to patients, the non-invasive photo-guided therapies are attracting massive attentions of researchers. Herein, the intelligent-designed carbon-dots/hemin nanoplatforms (HCDs NPs) were developed, owning high-authority photo-therapy for cancer. The fluorescence resonance energy transfer (FRET) effect enhanced the photo-thermal ability of HCDs NPs, endowing the synthesized nanoplatforms with photo-dynamic property simultaneously. Therefore, the obtained HCDs NPs could achieve synergetic photo-thermal and photo-dynamic therapies for cancer...
February 1, 2019: Journal of Inorganic Biochemistry
https://read.qxmd.com/read/30771672/photocatalytic-degradation-of-local-dyeing-wastewater-by-iodine-phosphorus-co-doped-tungsten-trioxide-nanocomposites-under-natural-sunlight-irradiation
#9
J O Tijani, O Ugochukwu, L A Fadipe, M T Bankole, A S Abdulkareem, W D Roos
In the present work, one-step green synthesis of WO3 based on the interaction of ammonium paratungstate and Spondias mombin leaves extract is reported. Different concentrations of iodine and phosphorus in the range of (2%, 5% and 10%) were firstly incorporated into the prepared WO3 nanoparticles to obtain Iodine doped and Phosphorus doped WO3 nanoparticles respectively. Subsequently, iodine and phosphorus co-doped WO3 nanocomposites was prepared using a wet impregnation method followed by calcination at high temperature...
February 13, 2019: Journal of Environmental Management
https://read.qxmd.com/read/30771082/voltammetric-simultaneous-determination-of-catechol-and-hydroquinone-using-a-glassy-carbon-electrode-modified-with-a-ternary-hybrid-material-composed-of-reduced-graphene-oxide-magnetite-nanoparticles-and-gold-nanoparticles
#10
Fen-Ying Kong, Rong-Fang Li, Lei Yao, Zhong-Xia Wang, Heng-Ye Li, Wei-Xin Lv, Wei Wang
An electrochemical sensor is described for the simultaneous determination of the pollutants catechol (CC) and hydroquinone (HQ). A glassy carbon electrode (GCE) was modified with reduced graphene oxide, Fe3 O4 and gold nanoparticles and then showed a pair of well-defined voltammetric peaks for CC and HQ. Its oxidation peak potentials (located at 0.21 and 0.10 V vs. Ag/AgCl) are well separated, and this makes it suitable for simultaneous determination of the two isomers. Under optimal conditions, the oxidation peak currents of CC and HQ increase linearly in the 0...
February 15, 2019: Mikrochimica Acta
https://read.qxmd.com/read/30765135/influence-of-graphene-oxide-and-biochar-on-anaerobic-degradation-of-petroleum-hydrocarbons
#11
Benru Song, Jingchun Tang, Meinan Zhen, Xiaomei Liu
The anaerobic degradation of petroleum is an important process in natural environments. So far, few studies have considered the response of the microbial community to nanomaterials during this process. This study explored the potential effects of graphene oxide and biochar on the anaerobic degradation of petroleum hydrocarbons in long-term experiments. Cyclic voltammetry and electrochemical impedance spectroscopy indicated that the addition of carbon-based materials promoted the electrochemical activity of anaerobic cultures that degrade petroleum hydrocarbons...
February 12, 2019: Journal of Bioscience and Bioengineering
https://read.qxmd.com/read/30761756/carbon-dots-in-matrix-boosting-intriguing-luminescence-properties-and-applications
#12
REVIEW
Jiyang Li, Bolun Wang, Hongyue Zhang, Jihong Yu
As a new class of luminescent nanomaterials, carbon dots (CDs) have aroused significant interest because of their fascinating photoluminescence properties and potential applications in biological, optoelectronic, and energy-related fields. Strikingly, embedding CDs in host matrices endow them with intriguing luminescent properties, in particular, room temperature phosphorescence and thermally activated delayed fluorescence, due to the confinement effect of the host matrix and the H-bonding interactions between CDs and the matrix...
February 13, 2019: Small
https://read.qxmd.com/read/30761748/water-dispersible-candle-soot-derived-carbon-nano-onion-clusters-for-imaging-guided-photothermal-cancer-therapy
#13
Wei Sun, Xiaodong Zhang, Hao-Ran Jia, Ya-Xuan Zhu, Yuxin Guo, Ge Gao, Yan-Hong Li, Fu-Gen Wu
Herein, water-dispersible carbon nano-onion clusters (CNOCs) with an average hydrodynamic size of ≈90 nm are prepared by simply sonicating candle soot in a mixture of oxidizing acid. The obtained CNOCs have high photothermal conversion efficiency (57.5%), excellent aqueous dispersibility (stable in water for more than a year without precipitation), and benign biocompatibility. After polyethylenimine (PEI) and poly(ethylene glycol) (PEG) modification, the resultant CNOCs-PEI-PEG have a high photothermal conversion efficiency (56...
February 14, 2019: Small
https://read.qxmd.com/read/30761622/3d-heteroatom-doped-carbon-nanomaterials-as-multifunctional-metal-free-catalysts-for-integrated-energy-devices
#14
REVIEW
Rajib Paul, Feng Du, Liming Dai, Yong Ding, Zhong Lin Wang, Fei Wei, Ajit Roy
Sustainable and cost-effective energy generation has become crucial for fulfilling present energy requirements. For this purpose, the development of cheap, scalable, efficient, and reliable catalysts is essential. Carbon-based heteroatom-doped, 3D, and mesoporous electrodes are very promising as catalysts for electrochemical energy conversion and storage. Various carbon allotropes doped with a variety of heteroatoms can be utilized for cost-effective mass production of electrode materials. 3D porous carbon electrodes provide multiple advantages, such as large surface area, maximized exposure to active sites, 3D conductive pathways for efficient electron transport, and porous channels to facilitate electrolyte diffusion...
February 14, 2019: Advanced Materials
https://read.qxmd.com/read/30761358/high-performance-supercapacitors-based-on-the-carbon-nanotubes-graphene-and-graphite-nanoparticles-electrodes
#15
L Fekri Aval, M Ghoranneviss, G Behzadi Pour
In this study, the three structures of the symmetric paper supercapacitors based on the carbon nanotubes (CNTs), graphite nanoparticles (GNPs) and graphene electrodes have been fabricated. In the supercapacitors was used of polyvinyl alcohol (PVA)/phosphoric acid (H3 PO4 ) as a gel electrolyte and the BaTiO3 film as a separator film. The carbon nanomaterials, gel electrolyte surface, and electrode films were characterized by scanning electron microscopy (SEM) and transmission electron microscope (TEM). The specific capacitance of the symmetric paper supercapacitors using charge-discharge technique and C-V curves at the voltage scan rates 20 mV/s and 150 mV/s have been investigated...
November 2018: Heliyon
https://read.qxmd.com/read/30758186/multi-color-raman-beads-for-multiplexed-tumor-cell-and-tissue-imaging-and-in-vivo-tumor-spectral-detection
#16
Qingqing Jin, Xinli Fan, Changmai Chen, Lei Huang, Jing Wang, XinJing Tang
Developing new nanomaterials with strong and distinctive Raman vibrations in the biological Raman-silent region (1800-2800 cm -1) were highly desirable for Raman hyper-spectral detection and imaging in living cells and animals. Herein, polymeric nanoparticles with monomers containing alkyne, cyanide, azide and carbon-deuterate were prepared as Raman-active nanomaterials (Raman Beads) for bioimag-ing applications. Intense Raman signals were obtained due to the high density of alkyne, cyanide, azide and carbon-deuterate in single nanoparticles, in absence of metal (such as Au or Ag) as Raman enhancers...
February 13, 2019: Analytical Chemistry
https://read.qxmd.com/read/30754027/novel-mesoporous-electrode-materials-for-symmetric-asymmetric-and-hybrid-supercapacitors
#17
Jayesh Cherusseri, Kowsik Sambath Kumar, Nitin Choudhary, Narasimha Nagaiah, Yeonwoong Jung, Tania Roy, Jayan Thomas
Electrochemical capacitors or supercapacitors have achieved great interest in the recent past due to their potential applications ranging from microelectronic devices to hybrid electric vehicles. Supercapacitors can provide high power densities but their inherently low energy density remains a great challenge. The high-performance supercapacitors utilize large electrode surface area for electrochemical double-layer capacitance and/or pseudocapacitance. To enhance the performance of supercapacitors, various strategies have been adopted such as electrode nanostructuring, hybrid electrode designs using nanocomposite electrodes and hybrid supercapacitor configurations...
February 12, 2019: Nanotechnology
https://read.qxmd.com/read/30746935/low-and-high-index-faceted-pd-nanocrystals-embedded-in-various-oxygen-deficient-wox-nanostructures-for-electrocatalytic-oxidation-of-alcohol-eoa-and-carbon-monoxide-co
#18
Karuppasamy Lakshmanan, Chin-Yi Chen, Sambandam Anandan, Jerry J Wu
This work suggests a modest hydrothermal method applied for the synthesis of oxygen-deficient WOx (x=2.75, 2.83, and 2.94) nanomaterial with various morphology, such as bundled nanorods (NR), nanobelts (NB), and nanosheets (NS), by changing the inorganic additives, such as HCl, NaHSO4, and HNO3. In addition, the WOx supported high and low index faceted Pd nanoparticles (Pd-WO2.75 NB, Pd-WO2.83 NR, and Pd-WO2.94 NS) have been successfully synthesized by the facile sonochemical method to function as the high-electrocatalytic activity of electrocatalysts for alcohol electrooxidation, including ethanol, ethylene glycol, and glycerol...
February 12, 2019: ACS Applied Materials & Interfaces
https://read.qxmd.com/read/30743910/impact-of-engineered-nanoparticles-on-microbial-transformations-of-carbon-nitrogen-and-phosphorus-in-wastewater-treatment-processes-a-review
#19
REVIEW
Shubiao Wu, Haiming Wu, Mark Button, Dennis Konnerup, Hans Brix
Concern regarding the potential negative impacts of released engineered nanoparticles (ENPs) on pollutant removal performance of wastewater treatment systems has received booming attention in recent years. However, the conclusions drawn from different studies often lead to fragmented overall knowledge, some of which are even contradictory. This scenario shows the necessity for a comprehensive review of the interactions of ENPs in wastewater treatment systems, particularly on the impacts of ENPs on microbial processes of carbon (C), nitrogen (N), and phosphorus (P) removal in water treatment systems...
April 10, 2019: Science of the Total Environment
https://read.qxmd.com/read/30741296/the-impact-of-tomato-fruits-containing-multi-walled-carbon-nanotube-residues-on-human-intestinal-epithelial-cell-barrier-function-and-intestinal-microbiome-composition
#20
Mohamed H Lahiani, Sangeeta Khare, Carl E Cerniglia, Ramiz Boy, Ilia N Ivanov, Mariya Khodakovskaya
Carbon nanomaterials (CNMs) can positively regulate seed germination and enhance plant growth. However, clarification of the impact of plant organs containing absorbed CNMs on animal and human health is a critical step of risk assessment for new nano-agro-technology. In this study, we have taken a comprehensive approach to studying the effect tomato fruits derived from plants exposed to multi-walled carbon nanotubes (CNTs) have on gastrointestinal epithelial barrier integrity and their impact on the human commensal intestinal microbiota using an in vitro cell culture and batch human fecal suspension models...
February 11, 2019: Nanoscale
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