Yongbiao Mu, Shixiang Yu, Yuzhu Chen, Youqi Chu, Buke Wu, Qing Zhang, Binbin Guo, Lingfeng Zou, Ruijie Zhang, Fenghua Yu, Meisheng Han, Meng Lin, Jinglei Yang, Jiaming Bai, Lin Zeng
Improving the long-term cycling stability and energy density of all-solid-state lithium (Li)-metal batteries (ASSLMBs) at room temperature is a severe challenge because of the notorious solid-solid interfacial contact loss and sluggish ion transport. Solid electrolytes are generally studied as two-dimensional (2D) structures with planar interfaces, showing limited interfacial contact and further resulting in unstable Li/electrolyte and cathode/electrolyte interfaces. Herein, three-dimensional (3D) architecturally designed composite solid electrolytes are developed with independently controlled structural factors using 3D printing processing and post-curing treatment...
January 12, 2024: Nano-Micro Letters